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  • 简介:Ultrafastfiberlasersareingreatdemandforvariousapplications,suchasopticalcommunication,spectroscopy,biomedicaldiagnosis,andindustrialfabrication.Here,wereportthehighlystablefemtosecondpulsegenerationfromaMXenemode-lockedfiberlaser.Wehavepreparedthehigh-qualityTi3C2Txnanosheetsviatheetchingmethod,andcharacterizedtheirultrafastdynamicsandbroadbandnonlinearopticalresponses.Theobviousintensity-andwavelength-dependentnonlinearresponseshavebeenobservedandinvestigated.Inaddition,ahighlystablefemtosecondfiberlaserwithsignal-to-noiseratioupto70.7dBandcentralwavelengthof1567.3nmhasbeendelivered.Thestudymayprovidesomevaluabledesignguidelinesforthedevelopmentofultrafast,broadbandnonlinearopticalmodulators,andopennewavenuestowardadvancedphotonicdevicesbasedonMXenes.

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  • 简介:利用天然气脱硫厂的酸气、氢氧化钠、对二氯苯和助剂磷酸钠,在六甲基苯磷酰三胺溶剂中,常压下缩聚4~6小时,制备了线型结晶性高分子量聚苯硫醚(HMWPPS)。该方法具有的明显优点是:设备简单、容易操作、活性高、溶剂稳定、产品收率高、成本低、适宜于大规模工业生产。

  • 标签: 高分子量聚苯硫醚 重复单元 切变粘度 六甲基磷酰三胺
  • 简介:MP3风靡我们的时候,我们就开始患上MP3疯魔症——眼睛睁开的第一秒,便搜索最爱的MP3,低头走路,孤立进食,默默无语……自始至终,活在一个人的世界里,你说,这不是疯了是怎么了?

  • 标签: MP3 设计 整机 电池
  • 简介:Afacilestep-by-stepapproachisdevelopedforsynthesizingthehigh-efficiencyandmagneticrecyclableFe_3O_4@SiO_2@Ag@Nitrepang-likenanocomposites.ThismethodinvolvescoatingFe_2O_3nanorodswithauniformsilicalayer,reductionin10%H_2/AratmospheretotransformtheFe_2O_3intomagneticFe_3O_4,andfinallydepositingAg@Nicore-shellnanoparticlesontheL-lysinemodifiedsurfaceofFe_3O_4@SiO_2nanorods.Thefabricatednanocompositesarefurthercharacterizedbyx-raydiffraction,transmissionelectronmicroscopy,scanningelectronmicroscope,Fouriertransforminfraredspectroscopy,andinductivelycoupledplasmamassspectroscopy.TheFe_3O_4@SiO_2@Ag@Nitrepang-likenanocompositesexhibitremarkablyhighercatalyticefficiencythanmonometallicFe_3O_4@SiO_2@AgnanocompositestowardthedegradationofRhodamineB(RhB)atroomtemperature,andmaintainsuperiorcatalyticactivityevenaftersixcycles.Inaddition,thesesamplescouldbeeasilyseparatedfromthecatalyticsystembyanexternalmagnetandreused,whichshowsgreatpotentialapplicationsintreatingwastewater.

  • 标签: 纳米复合材料 降解效率 催化剂 可回收 有机染料 海参
  • 简介:High-performancethin-filmtransistors(TFTs)withalowthermalbudgetarehighlydesiredforflexibleelectronicapplications.Inthiswork,theTFTswithatomiclayerdepositedZnO-channel/Al_2O_3-dielectricarefabricatedunderthemaximumprocesstemperatureof200℃.First,weinvestigatetheeffectofpost-annealingenvironmentsuchasN_2,H_2-N_2(4%)andO_2onthedeviceperformance,revealingthatO_2annealingcangreatlyenhancethedeviceperformance.Further,wecomparetheinfluencesofannealingtemperatureandtimeonthedeviceperformance.Itisfoundthatlongannealingat200℃isequivalenttoandevenoutperformsshortannealingat300℃.ExcellentelectricalcharacteristicsoftheTFTsaredemonstratedafterO_2annealingat200℃for35min,includingalowoff-currentof2.3×10~(-13)A,asmallsub-thresholdswingof245mV/dec,alargeon/offcurrentratioof7.6×10~8,andahighelectroneffectivemobilityof22.1cm~2/V·s.Undernegativegatebiasstressat—10V,theabovedevicesshowbetterelectricalstabilitiesthanthosepost-annealedat300℃.Thusthefabricatedhigh-performanceZnOTFTwithalowthermalbudgetisverypromisingforflexibleelectronicapplications.

  • 标签: 薄膜晶体管 退火温度 原子层沉积 通道 电特性 氧化铝
  • 简介:当堂反馈1.压强是反映——的物理量.一辆“东风牌”汽车对地面的压强是1.8×10^4Pa它所表示的物理含义是——.

  • 标签: 压强 物理量 东风牌
  • 简介:通过软件实现了用PC机调用日本Rigaku公司生产的D/max一类X射线衍射仪测量数据,利用PC机的复杂计算功能,使原有仪器也可以进行新的结构分析工作,扩展了仪器的功能。

  • 标签: X射线结构分析 软件 数据处理
  • 简介:小角X射线散射(SAXS)是研究多孔材料结构的一种有效方法.可得到孔径分布、平均孔径、比表面、界面层厚度、分形维数等许多微结构信息.SAXS理论公式基于点状光源(针孔准直),但实践中则大多采用长狭缝准直条件.简要综述了SAXS在长狭缝准直条件下直接应用模糊强度进行煤、炭、二凝胶、分子筛等多孔材料结构解析的方法、并与针孔准直进行了对比。

  • 标签: 小角X射线散射 多孔材料 模糊数据 结构分析 解析方法 SAXS
  • 简介:Inthefarfieldoftheintensitydistributionofthebeamdeliveredbyatwo-stagetransient–collisionalexcitationX-raylaser(XRL),anon-expectedinterferencepatternthatisstablefromshottoshothasbeendiscovered.Itisdemonstratedthattheinterferenceiscausedbytheemergenceofanimaginarysourceintheamplifyingplasma,whichisphasematchedtotheradiationofthegenerator.TheobservedphenomenoniscalledanX-raycoherentmirage.Toexplaintheobtainedresults,anewtheoreticalapproachisdeveloped.ThebasicessentialconditionsforformationoftheX-raymirageareformulated,andpossibleapplicationsarediscussed.Thispaperdetailstheexperiments,includingtheformulationofthenecessaryandsufficientconditionsforformationoftheX-raymirage,andpossibleapplicationsarediscussed.

  • 标签: COHERENT seeded BEAMS MIRAGE PHASE-MATCHING X-RAY
  • 简介:ThestatusoftheEuropeanX-rayFree-ElectronLaser(EuropeanXFEL),underconstructionnearHamburg,Germany,isdescribed.ThestartofoperationsoftheLCLSatSLACandofSACLAinJapanhasalreadyproducedimpressivescientificresults.TheEuropeanXFELfacilityispoweredbya17.5GeVsuperconductinglinearacceleratorthat,comparedtothesetwooperatingfacilities,willgeneratetwoordersofmagnitudemorepulsespersecond,upto27000.Itcanthereforesupportmodesofoperationswitchingthebeamupto30timespersecondamongthreedifferentexperiments,providingeachofthemwiththousandsofpulsespersecond.Thescientificpossibilitiesopenedupbythesecapabilitiesarebrieflydescribed,togetherwiththecurrentinstrumentaldevelopments(inoptics,detectors,lasers,etc.)thatarenecessarytoimplementthisprogram.

  • 标签: FEMTOSECOND LASERS and APPLICATIONS free-electron LASERS
  • 简介:研究了钙钛矿太阳能电池材料CH3NH3PbI3(CH3NH3=MA,MAPbI3)的输运特性,理论分析了有机分子MA对晶格结构的影响。发现:MA沿[110]方向排布且近邻MA分子相互垂直的构型最稳定,将此构型作为MAPbI3的标准结构,使用第一性原理方法,通过分析晶格的振动散射或声子散射,计算了MAPbI3材料中形变势散射主导的载流子迁移率,分析了材料的输运特性,讨论了载流子迁移率理论计算值和实验值之间的差异。

  • 标签: CH3NH3PbI3 几何结构 形变势散射 迁移率
  • 简介:YbxY1-xAl3(BO3)4(x=0.1,0.07and0)crystalshavebeengrownbythefluxmethod.ThegrowthdefectsofYbxY1-xAl3(BO3)4crystalsweredetectedbyX-raytopography.ItisfoundthattheperfcetionofYbYABcrystalwithlowYbdopantisbetterthanthatwithhighYbdopant.InYb0.1Y0.9Al3(BO3)4crystal,growhtbands,growthboundaries,grown-indislocationsandinclusionswereobserved.Howver,thedensitiesofgrowthdefectsforYb0.07Y0.93Al3(BO3)4andYAl3(BO3)4arelowandnoobviousinclusionsareobservedinthesecrytals.Inaddition,growthtwinswrerdetectedinYbxY1-xAl3(BO3)4crystalbyusingthechemicaletchingmethod.ItisfoundthatthegrowthtwinsoccurfrequentlyinYb0.01Y0.9Al3(BO3)4crystalwhereasnogrowthtwinappearsinYAl3(BO3)4crystal.Basedontheexperimentalobservations,theformationmechanismofgrowthtwinsisdiscussed.Inthemeantime,theeffectivemeasuresforreducingthegrowthtwinsanddefectsareproposed.2001ElsevierScienceB.V.Allrightsreserved.

  • 标签: YbxY1-xAl3(BO3)4晶体 晶体生长 结构缺陷 硼酸盐晶体 形貌学 X射线
  • 简介:目的:探索燃料富氧燃烧过程中不同浓度CO2的稀释作用对NOx生成的影响,为探索Nx在O2/CO2气氛中生成机理研究提供理论基础。创新点:提出一种无分支链式反应解释说明CO2在还原性粒子环境中对反应的影响。方法:通过ChemkinPro中塞流式反应器模块对混入NH3的CH4燃料在O2/CO2气氛中反应进行数值模拟,同时改变CO2的稀释程度来探索CO2浓度对NOx生成的影响,并比较不同反应机理下的模拟结果,探索此环境中NOx的生成机理(表1)。结论:1.无支链反应机理可用于解释CO2在还原性粒子环境中对Nq生成与还原的影响;2.随着C02浓度的升高,无支链反应和支链反应相互竞争H,进而抑制NO的生成;3.在对NH,转化效率的影响方面,CO2浓度增加引发的无支链反应和支链反应对H的竞争,在富燃料条件下从促进转化变为抑制转化,在化学当量和贫燃料条件下从无影响变为抑制转化。

  • 标签: CO2 富氧燃烧 NO 燃料稀释
  • 简介:Inthispaper,weproposealocalfuzzymethodbasedontheideaof"p-strong"communitytodetectthedisjointandoverlappingcommunitiesinnetworks.Inthemethod,arefinedagglomerationruleisdesignedforagglomeratingnodesintolocalcommunities,andtheoverlappingnodesaredetectedbasedontheideaofmakingeachcommunitystrong.Weproposeacontributioncoefficientbvcitomeasurethecontributionofanoverlappingnodetoeachofitsbelongingcommunities,andthefuzzycoefficientsoftheoverlappingnodecanbeobtainedbynormalizingthebvcitoallitsbelongingcommunities.Therunningtimeofourmethodisanalyzedandvarieslinearlywithnetworksize.Weinvestigateourmethodonthecomputergeneratednetworksandrealnetworks.Thetestingresultsindicatethattheaccuracyofourmethodindetectingdisjointcommunitiesishigherthanthoseoftheexistinglocalmethodsandourmethodisefficientfordetectingtheoverlappingnodeswithfuzzycoefficients.Furthermore,thelocaloptimizingschemeusedinourmethodallowsustopartlysolvetheresolutionproblemoftheglobalmodularity.

  • 标签: 检测网络 模糊方法 社区 模糊系数 计算机网络 网络规模