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53 个结果
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  • 简介:Ultrafast各向异性的腐烂是揭示ultrafast精力和电子转移的一个突出的参数;然而,由于平行和垂直极化的腐烂动力学的同时的可获得性的要求可靠地坚定是困难的。现在,各向异性的腐烂的任何测量是准确同时性的一种途径。这里,我们为同步ultrafastanisotropy腐烂大小报导一个新奇方法,它能很好决定anisotropy,甚至在一很早的时间,作为刺激激光脉搏的升起的阶段。在与协调刺激在房间温度在答案收获Rhodobactersphaeroides的天线建筑群LH2的细菌的光的B850的各向异性的腐烂被这个方法检测,它显示出30fs的一极化反应时间,并且到在B850戒指的bacteriochlorophylls的从起始的刺激的精力转移拿大约70fs。在吸收光谱的红方面被探查的各向异性的腐烂例如880nm,有0.4的起始的价值,相应于模仿的排放,当有0.1的anisotropy的蓝方面贡献漂白的地面状态时。我们的结果证明盖住整个戒指的协调刺激可能没由于LH2碎的对称被认识到:从在到在答案的C2对称的膜的C9对称。

  • 标签: 各向异性 同步测量 LH2 复合物 细菌 衰减动力学
  • 简介:Thereisagrowingsupportforthelowlyingscalarmesonsf0(500),f0(980),a0(980),and(800)tobegenerateddynamicallyfromtheinteractionofpseudoscalarmesons,whilethecaseofthenextsetofscalarresonancesathigherenergies,f0(1370),f0(1710),K0(1430)ismoreaquestionofdebate.Soisthecaseofthetensorresonancesf2(1270),f′2(1525),K2(1430).AnewperspectiveonthesestateshasbeenofferedinRef.[1]wherethef0(1370)andf2(1270)resonancesareshowntobegeneratedfromtheinteractionprovidedbythelocalhiddengaugeLagrangiansimplementingunitarization.Itisshownthattheideaofthenatureofthesestatesasvectormeson-vectormesoncompositestateshasbeentestedinmanyreactions.Yet,thepermanentdiscussionoftheissuedemandsextrachecksforotherobservablesand,inthissense,theweakdecaysbringanewsourceofvaluableinformationthatshouldservetotestdifferentmodels.

  • 标签: J/Ψ source case SENSE NEXT IDEA
  • 简介:Inthispaper,blendmembranesfrompolyvinylacetate(PVAc)andblockcopolymerpoly(amide-12-b-ethyleneoxide)(Pebax1074)arepreparedbysolutioncastingandsolventevaporationmethod.Althoughtheyarehomogeneousonamacro-scale,theobservationsfromDSCandSEMindicatemicro-phaseseparationforPVAc/Pebax1074blendmembranes.WiththeincreaseofPebax1074content,gaspermeabilitiesofCO2,H2,N2andCH4allincreasegreatly.PVAc/Pebax1074blendmembraneswithhighPVAccontentareappropriateforCO2/CH4separation.Thetemperaturedependenceofgaspermeabilityisdividedintorubberyregionandglassyregion.Theactivationenergiesofpermeationinrubberyregionaresmallerthanthoseinglassyregion,andtheyalldecreasewithincreasingPebax1074content.ForN2,H2andCH4,theirgaspermeationpropertiesaremainlyinfluencedbythedual-modesorptionandhydrostaticpressureeffect.ButforCO2,itspermeabilityincreaseswiththeincreaseofpressureduetoCO2-inducedplasticizationeffect,whichismoreobviousforPVAc/Pebax1074blendmembraneswithhighPVAccontent.

  • 标签: polyvinyl acetate poly(amide-12-b-ethylene oxide) blend membrane
  • 简介:Inthisarticle,wecalculatethecontributionfromthenonfactorizablesofthadronicmatrixelementtothedecayB~0→χc1~π~0withthelight-conequantumchromo-dynamic(QCD)sumrules.Thenumericalresultsshowthatitscontributionisratherlargeandshouldnotbeneglected.Thetotalamplitudesleadtoabranchingfractionwhichisinagreementwiththeexperimentaldatamarginally.

  • 标签: QCD求和规则 衰变 计算结果 强子矩阵元 实验数据 动力学
  • 简介:Thermoelectricityisatherrnorelatedpropertythatisofgreatimportanceinsingle-moleculejunctions.Theelectricalconductance(σ),electron-derivedthermalconductance(kel)andSeebeckcoefficient(S)ofBgo-basedsingle-moleculejunctionsareinvestigatedbyusingdensityfunctionaltheoryincombinationwithnon-equilibriumGreen'sfunction.Whenthedistancebetweentheleft/rightelectrodesis11.4A,therelationshipbetweenσandkelobeystheWiedemann-FranzlawverywellbecauseofthestronghybridizationbetweenB80molecularorbitalsandthesurfacestatesofAuelectrodes.Furthermore,thecalculatedLorenznumberisclosetothefamousvalueinmetalordegeneratesemiconductors.Inaddition,Sisonly—19.09μV/Kat300K,thusleadingtothesmallerelectron'sthermoelectriefigureofmerit(ZeiT=S^2σT/Kel).Interestingly,thestrainandchemicalpotentialcanmodulateB80-basedsingle-moleculejunctionsfromn-typetop-typewhenthecompressivestrainreaches—0.6Aorthechemicalpotentialshiftsto—0.16eV.ThismightbeattributedthatSreflectstheasymmetryintheelectricalconductancewithrespecttothechemicalpotentialandisproportionaltotheslopesofthetransmissionspectrum.

  • 标签: THERMOELECTRICITY SINGLE-MOLECULE JUNCTION NON-EQUILIBRIUM Green FUNCTION
  • 简介:Theoreticalmodelsofstellarevolutionpredictnegligiblequantitiesof6Li,9Be,and11Binthehydrogenburningphasesofastar’sevolution[1].TheprimordialBig-Bangnucleosynthesis(BBN)modelmightbemoregenerousinitsproductionoftheseelements[2].Theradiative-capturecrosssectionforprotoncaptureon11Bleadingto12CissmallatastrophysicallyinterestingenergiesbecauseofthelargeCoulombbarrier.

  • 标签: FACTORS LOW ENERGIES
  • 简介:Underinvestigationinthispaperisa(3+1)-dimensionalvariable-coefficientKadomtsev–Petviashviliequation,whichdescribesthepropagationofsurfaceandinternalwaterwaves.ByvirtueofthebinaryBellpolynomials,symboliccomputationandauxiliaryindependentvariable,thebilinearforms,solitonsolutions,B¨acklundtransformationsandLaxpairareobtained.Variablecoefficientsoftheequationcanaffectthesolitonicstructure,whentheyarespeciallychosen,whilecurvedandlinearsolitonsareillustrated.Elasticcollisionsbetween/amongtwoandthreesolitonsarediscussed,throughwhichthesolitonskeeptheiroriginalshapesinvariantexceptforsomephaseshifts.

  • 标签: LAX对 变系数 孤立波解 方程 BACKLUND变换 双线性形式