The mechanism of the UV band edge photorefractivity suppression in highly doped LiNbO3:Zr crystals

(整期优先)网络出版时间:2017-06-16
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Theultraviolet(UV)bandedgephotorefractivityofLiNbO_3:Zrat325nmhasbeeninvestigated.Theexperimentalresultsshowthattheresistanceagainstphotorefractionat325nmisquiteobviousbutnotasstrongasthatat351nm,whenthedopingconcentrationofZrreaches2.0mol%.ItisreportedthatthephotorefractivityinothertetravalentlydopedLiNbO_3crystals,suchasLiNbO_3:HfandLiNbO_3:Sn,isenhanceddramaticallywithdopingconcentrationoverthreshold.HerewegiveanexplicitexplanationonsuchseemlyconflictingbehaviorsoftetravalentlydopedLiNbO_3,whichisascribedtothecombinedeffectofincreasedphotoconductivityandtheabsorptionstrengthofthebandedgephotorefractivecenters.