简介:Westudypreconditioningtechniquesusedinconjunctionwiththeconjugategradientmethodforsolvingmulti-length-scalesymmetricpositivedefinitelinearsystemsoriginatingfromthequantumMonteCarlosimulationofelectroninteractionofcorrelatedmaterials.Existingpreconditioningtechniquesarenotdesignedtobeadaptivetovaryingnumericalpropertiesofthemulti-length-scalesystems.Inthispaper,weproposeahybridincompleteCholesky(HIC)preconditioneranddemonstrateitsadaptivitytothemulti-length-scalesystems.Inaddition,weproposeanextensionofthecompressedsparsecolumnwithrowaccess(CSCR)sparsematrixstorageformattoefficientlyaccommodatethedataaccesspatterntocomputetheHICpreconditioner.Weshowthatformoderatelycorrelatedmaterials,theHICpreconditionerachievestheoptimallinearscalingofthesimulation.Thedevelopmentofalinear-scalingpreconditionerforstronglycorrelatedmaterialsremainsanopentopic.
简介:最近,大努力在任意的弄歪的设备的制造被作了满足便携、小的电子产品的要求。当它是一个很挑战性的工作时,灵活底层上的高水晶的优秀电影的直接生长是最理想的方法与当前的半导体设备由于简单、兼容的准备技术的优点制作灵活设备,并且通常非结晶、多晶或不连续的单个水晶的电影被完成。这里,我们表明高质量的双性人2Te3单身者由修改的热墙取向附生技术的灵活polyimide底层上的水晶的电影。试验性的结果表明邻近的雏晶协调地被联合形成一部连续电影,尽管迷惑的雏晶的数量由于快生长率被产生。由把一个石英过滤器插入到生长试管,迷惑的雏晶的数字密度有效地由于改进螺线相互作用被减少。而且,灵活双性人2Te3光电导体被制作并且在弯曲的不同的度下面展出强壮的在红外线附近的光导的反应,它也证实对电子应用合适的获得的灵活电影。
简介:Thestrategyofsequentiallyspin-coatingaperovskitefilmfromtheperovskiteprecursorandanelectrontransportinglayerof[6,6]-phenyl-C71-butyricacidmethylester(PC71BM)isdevelopedtosimplifythefabricationprocedureofperovskitesolarcells.X-raydiffractionandscanningelectronmicroscopyindicatethatPC71BMfilmonperovskitelayercanretardtheevaporationofdimethylsulfoxide(DMSO)efficiently,thusprolongingthetransformationofintermediatephasetoperovskitecrystals,leadingtoahighqualityperovskitethinfilm.Thesolarcellswiththestructureofindiumtinoxides(ITO)/poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate)(PEDOT:PSS)/CH3NH3PbI3/PC71BM/bathocuproine(BCP)/Agmadefromthissimplifiedmethodexhibitahigherefficiency(12.68%)thanthosefromtheconventionalone-stepmethod(9.49%).
简介:A100-J-levelNd:glasslasersysteminnanosecond-scalepulsewidthhasbeenconstructedtoperformasastandardsourceofhigh-fluence-laserscienceexperiments.Thelasersystem,operatingwithtypicalpulsedurationsof3–5nsandbeamdiameter60mm,employsasequenceofsuccessiverodamplifierstoachieve100-J-levelenergyat1053nmat3ns.Thefrequencyconversioncanprovideenergyof50-Jlevelat351nm.Inadditiontothehighstabilityoftheenergyoutput,themostvaluableofthelasersystemisthehighspatiotemporalbeamqualityoftheoutput,whichcontainstheuniformsquarepulsewaveform,theuniformflat-topspatialfluencedistributionandtheuniformflat-topwavefront.
简介:Fractionalpyrolysisandone-steppyrolysisofnaturalalgaeCyanobacteriafromTaihuLakewerecomparativelystudiedfrom200to500°C.One-steppyrolysisproducedbio-oilwithcomplexcompositionandlowhighheatingvalue(HHV30.9MJ/kg).FractionalpyrolysisseparatedthedegradationofdifferentcomponentsinCyanobacteriaandimprovedtheselectivitytoproductsinbio-oil.Thatis,acidsat200°C,amidesandacidsat300°C,phenolsandnitrilesat400°C,andphenolsat500°C,weregotasmainproducts,respectively.HZSM-5couldpromotethedehydration,crackingandaromatizationofpyrolyticintermediatesinfractionalpyrolysis.AtoptimalHZSM-5catalystdosageof1.0g,theselectivitytoproductsandthequalityofbio-oilwereimprovedobviously.Themainproductsinbio-oilchangedtonitriles(47.2%)at300°C,indoles(51.3%)andphenols(36.3%)at400°C.Theoxygencontentwasreducedto7.2wt%and9.4wt%,andtheHHVwasraisedto38.1and37.3MJ/kgat300and400°C,respectively.Fractionalcatalyticpyrolysiswasproposedtobeanefficientmethodnotonlytoprovideapotentialsolutionforalleviatingenvironmentalpressurefromwaterblooms,butalsotoimprovetheselectivitytoproductsandobtainhighqualitybio-oil.
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简介:Wereportontheperformanceofacontinuous-waveNd:GdVO4laserin-banddiode-pumpedat912nmwithhighoutputpowerandexcellentbeamquality.Thelaserproducedanoutputpowerof19.8Wat1063nmwithanopticalefficiencyof59.3%andslopeefficiencyof62.7%.Thelaserthresholdwas2.04Woftheabsorbedpumppower,andthelaseroutputbeamqualitywas≤1.2inthehorizontalandverticaldirections.Thestrengthofthermallensingatfulloutputpower(33.4Wofabsorbedpower)wasmeasuredtobeanaverageof8.6diopters.Itisshownthatthermallensingisreducedbyafactorof2withrespecttotheNd:YVO4lasers,thusopeningawayforfurtheroutput-powerscaling.
简介:Wehavesuccessfullydemonstratedthathighqualityandhighdielectricconstantlayerscanbefabricatedbylowtemperaturephoto-inducedor-assistedprocessing.Ta2O5andZrO2havebeendepositedatt<400℃bymeansofaUVphoto-CVDtechniqueandHfO2byphoto-assistedsol-gelprocessingwiththeaidofexcimerlamps.TheUVannealingofas-grownlayerswasfoundtosignificantlyimprovetheirelectricalproperties.Lowleakagecurrentdensitiesontheorderof10-8A/cm2at1MV/cmfordepositedultrathinTa2O5filmsandca.10-6A/cm2forthephoto-CVDZrO2layersandphoto-irradiatedsol-gelHfO2layershavebeenreadilyachieved.TheimprovementintheleakagepropertiesoftheselayersisattributedtotheUV-generatedactiveoxygenspeciesO(1D)whichstronglyoxidizeanysuboxidestoformmorestoichiometricoxidesonremovingcertaindefects,oxygenvacanciesandimpuritiespresentintheas-preparedlayers.Thephoto-CVDTa2O5filmsdepositedacross10.16-cmSiwafersexhibitahighthicknessuniformitywithavariationoflessthan±2.0%beingobtainedforultrathinca.10nmthickfilms.Thelamptechnologycaninprinciplebeextendedtolargerareawafers,providingapromisinglowtemperatureroutetothefabricationofarangeofhighqualitythinfilmsforfutureULSItechnology.