Efficient oxidation of ethylbenzene catalyzed by cobalt zeolitic imidazolate framework ZIF-67 and NHPI-中国期刊网

摘要 EfficientcatalyticoxidationofethylbenzenetoacetophenonewasrealizedusingthecatalyticsystemofcobaltzeoliticimidazolateframeworkZIF-67/N-hydroxyphthalimide(NHPI)undermildconditions.95.2%conversionofethylbenzenewith90.3%selectivitytoacetophenonecouldbeobtainedat373Kunder0.3MPaO2for9h.TheresultsshowthatthereexistssynergeticeffectbetweenZIF-67andNHPI.1-Phenylethylhydroperoxide(PEHP)wasgeneratedviaaradicalprocessinvolvingthehydrogenabstractionfromethylbenzenebyphthalimideN-oxyl,andsubsequentlyeffectivelydecomposedtoacetophenonebyZIF-67.

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Efficient oxidation of ethylbenzene catalyzed by cobalt zeolitic imidazolate framework ZIF-67 and NHPI

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Efficient oxidation of ethylbenzene catalyzed by cobalt zeolitic imidazolate framework ZIF-67 and NHPI

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